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Shear viscosity of slightly-elastic concentrated suspensions at low and high shear rates
Authors:Maw-Ling Wang  Tei-Chih Cheau
Affiliation:1. Department of Chemical Engineering, National Tsing Hua University, 30043, Hsinchu, Taiwan, ROC
Abstract:A quasi-static asymptotic analysis is employed to investigate the elastic effects of fluids on the shear viscosity of highly concentrated suspensions at low and high shear rates. First a brief discussion is presented on the difference between a quasi-static analysis and the periodic-dynamic approach. The critical point is based on the different order-of-contact time between particles. By considering the motions between a particle withN near contact point particles in a two-dimensional “cell” structure and incorporating the concept of shear-dependent maximum packing fraction reveals the structural evolution of the suspension under shear and a newly asymptotic framework is devised. In order to separate the influence of different elastic mechanisms, the second-order Rivlin-Ericksen fluid assumption for describing normal-stress coefficients at low shear rates and Harnoy's constitutive equation for accounting for the stress relaxation mechanism at high shear rates are employed. The derived formulation shows that the relative shear viscosity is characterized by a recoverable shear strain,S R at low shear rates if the second normal-stress difference can be neglected, and Deborah number,De, at high shear rates. The predicted values of the viscosities increase withS R , but decrease withDe. The role ofS R in the matrix is more pronounced than that ofDe. These tendencies are significant when the maximum packing fraction is considered to be shear-dependent. The results are consistent with that of Frankel and Acrivos in the case of a Newtonian suspension, except for when the different divergent threshhold is given as [1 ? (Φ/Φ m )1/2] ? 1.
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