Silver-catalyzed cycloisomerization of 1,n-allenynamides |
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Authors: | Garcia Pierre Harrak Youssef Diab Lisa Cordier Pierre Ollivier Cyril Gandon Vincent Malacria Max Fensterbank Louis Aubert Corinne |
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Affiliation: | UPMC Universite? Paris 06, Sorbonne Universite?s, Institut Parisien de Chimie Mole?culaire (UMR CNRS 7201), Paris, France. |
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Abstract: | A variety of allenynamides can undergo cycloisomerization reactions in the presence of silver triflate thus leading to the formation of N-containing heterocycles incorporating cross-conjugated trienes. Access to new dienic 4-piperidinone and azepane motifs was achieved. An extension to one-pot tandem sequences involving silver-catalyzed cycloisomerization/Diels-Alder reaction was also examined. |
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