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Stark-enhanced diode-laser spectroscopy of formaldehyde using a modified Herriott-type multipass cell |
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| Authors: | C. Dyroff P. Weibring A. Fried D. Richter J.G. Walega A. Zahn W. Freude P. Werle |
| Affiliation: | 1. Institute for Meteorology and Climate Research, Research Center Karlsruhe, Hermann-von-Helmholtz-Platz 1, 76344, Eggenstein-Leopoldshafen, Germany 2. Earth Observing Laboratory, National Center for Atmospheric Research, 3450 Mitchell Lane, Boulder, CO, 80301, USA 3. Institute of High-Frequency and Quantum Electronics, Universit?t Karlsruhe (TH), Engesserstrasse 5, 76131, Karlsruhe, Germany 4. CNR-National Institute for Applied Optics, Largo E. Fermi, 6, 50125, Florence, Italy |
| Abstract: | The combined use of a novel multipass cell and a sample modulation scheme based on the Stark effect in molecular spectra is used to suppress time dependent background signals, which in general limit spectrometer performance during measurements. A rapid background subtraction scheme, in which the external electric field was turned off on alternate scans, as well as a double modulation experiment show drift free, white noise limited characteristics up to integration times of more than 1000 s. This exceeds the generally obtained spectrometer stability by about one order of magnitude. PACS 82.80.Gk; 42.62.Fi; 07.88.+y; 33.55.Be |
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