Critical thermodynamics of dysprosium ethyl sulphate,a pure dipolar Ising ferromagnet

Using a SQUID magnetometer the magnetization of the Ising ferromagnet dysprosium ethyl sulphate has been measured in the temperature range 0.015–3K and in external fields 0.004–30 Oe. The results atT0.4 K (precritical regime) confirm the pure dipolar nature of the magnetic interactions. Particular interest has been paid to the immediate neighbourhood of the critical pointT _c =118.17 mK andH=0 where the zero-field susceptibility(T) aboveT _c , the spontaneous magnetizationM _s (T), and the magnetization atT _c ,M _c (H), can be described by mean field laws modified by logarithmic singularities. The critical amplitudes, B, andD of, M _s andM _c , respectively, satisfy the relation (2/3B ²)^1/3=D. All these results agree with predictions of (i) the Larkin-Khmel'nitskii theory and (ii) exact solutions of the renormalization group equations for 3-dimensional dipolar Ising ferromagnets.A project of the Sonderforschungsbereich 65 Festkörperspektroskopie Darmstadt-Frankfurt, financed by special funds of the Deutsche Forschungsgemeinschaft