Multiphoton ion pair spectroscopy (MPIPS) with ultrashort laser pulses for the H2 molecule |
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Authors: | Bandrauk André D Tchitchekova Deyana S Chelkowski Szczepan |
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Institution: | Laboratoire de Chimie Théorique, Département de Chimie, Faculté des Sciences, Université de Sherbrooke, Sherbrooke, Québec J1K 2R1, Canada. Andre.Bandrauk@USherbrooke.ca |
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Abstract: | Time-dependent Schr?dinger equation, TDSE, simulations have been performed in order to prepare and study via MPIPS the evolution of vibrational wave packets on the ion pair electronic state potentials B'B1Sigma(u)(+) and Hh1Sigma(g)(+) of the H2 molecule. Using ab initio potential surfaces and transition moments, we present two- and three-photon excitation schemes with ultrashort pulses (tau
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