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Influence of the vibrational quantum number of the resonant state in resonant multiphoton ionization/dissociation of hydrogen molecules
Affiliation:Association EURATOM- FOM, FOM Institute for Atomic and Molecular Physics, Kruislaan 407, 1098 SJ Amsterdam, The Netherlands;School of Physics, Dalian University of Technology, Dalian 116024, China;Department of Emergency Medicine, University of California San Diego Health System, San Diego, California
Abstract:We have studied the resonant multiphoton ionization of hydrogen in a three-photon excitation, one-photon ionization scheme. Superimposed on the ionization process we find a dissociation mechanism which manifests itself in a strong H+ signal. The ratio of H+ to H+2 signals depends on the vibrational quantum number v' of the intermediate state and on the laser intensity. We present a simple model which qualitatively reflects this dependence.
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