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Three-dimensional photon confinement in a spherical microcavity with CdTe quantum dots: Raman spectroscopy
Authors:YuP Rakovich  M Gerlach  JF Donegan  N Gaponik  AL Rogach
Institution:aSemiconductor Photonics Group, Department of Physics, Trinity College, Dublin 2, Ireland;bInstitute of Physical Chemistry, University of Hamburg, 20146 Hamburg, Germany;cDepartment of Physics and CeNS, Ludwig-Maximilians-Universität München, 80799 Munich, Germany
Abstract:We have studied the Raman spectra of a system consisting of a polystyrene latex microsphere coated by CdTe colloidal quantum dots. The cavity-induced enhancement of the Raman scattering allows the observation of Raman spectra from only one CdTe monolayer. Periodic structure with very narrow peaks in the Raman spectra of a single microsphere was detected both in Stokes and anti-Stokes spectral regions, arising from the coupling between the emission from quantum dots and spherical cavity modes.
Keywords:Raman scattering  Spherical microcavity  Nanocrystals
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