High-frequency dielectric study of the dynamics of (KBr)1−x (KCN) x mixed crystals |
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Authors: | J. F. Berret P. Doussineau A. Levelut W. Schön |
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Affiliation: | (1) Laboratoire de Science des Matériaux Vitreux, Université des Sciences et Techniques du Languedoc, F-34060 Montpellier, France;(2) Laboratoire d'Ultrasons, Université Pierre et Marie Curie, F-75252 Paris, France |
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Abstract: | Dielectric measurements have been performed at 1 and 10 GHz in (KBr)1–x(KCN)x mixed crystals for cyanide concentrationsx=0.25 andx=0.50 in the temperature rangeT=1.7–150 K. The maxima of the real and imaginary parts of the dielectric constant falls into the Arrhenius straight lines obtained at lower frequencies. These dipolar lines cross over the so-called quadrupolar (acoustic) lines, in contradiction with theoretical predictions on the nature of the freezing. We also present a qualitative model which reinterprets the dipolar and quadrupolar freezings in terms of an individual and a collective processes.Associated with the Centre National de la Recherche Scientifique |
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