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3-D composite electrodes for high performance PEM fuel cells composed of Pt supported on nitrogen-doped carbon nanotubes grown on carbon paper
Authors:Madhu Sudan Saha  Ruying Li  Xueliang Sun  Siyu Ye
Institution:1. Department of Mechanical and Materials Engineering, The University of Western Ontario, London, Ontario, Canada N6A 5B9;2. Ballard Power Systems Inc., 9000 Glenlyon Parkway, Burnaby, BC, Canada V5J 5J8
Abstract:The 3-D composite electrodes consisting of Pt nanoparticles supported on nitrogen-doped carbon nanotubes (CNx) grown directly on carbon paper were successfully prepared. The effect of the nitrogen atom incorporation in carbon nanotubes (CNTs) on the Pt nanoparticle dispersion and catalytic activities for the oxygen reduction reaction has been investigated. Compared to regular CNTs, highly dispersed Pt nanoparticles with smaller size (2–3 nm) and higher electrochemical Pt surface area as well as higher fuel cell performance were obtained for CNx.
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