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beta-NMR of isolated lithium in nearly ferromagnetic palladium
Authors:Parolin T J  Salman Z  Chakhalian J  Song Q  Chow K H  Hossain M D  Keeler T A  Kiefl R F  Kreitzman S R  Levy C D P  Miller R I  Morris G D  Pearson M R  Saadaoui H  Wang D  MacFarlane W A
Institution:Department of Chemistry, University of British Columbia, Vancouver, BC, V6T 1Z1, Canada.
Abstract:The temperature dependence of the frequency shift and spin-lattice relaxation rate of isolated, nonmagnetic (8)Li impurities implanted in a nearly ferromagnetic host (Pd) are measured by means of beta-detected nuclear magnetic resonance (beta-NMR). The shift is negative, very large, and increases monotonically with decreasing T in proportion to the bulk susceptibility of Pd for T > T* approximately 100 K. Below T*, an additional shift occurs which we attribute to the response of Pd to the defect. The relaxation rate is much slower than expected for the large shift and is linear with T below T*, showing no sign of additional relaxation mechanisms associated with the defect.
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