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Dynamic fluctuations and static speckle in critical X-ray scattering from SrTiO3
Authors:Holt M  Sutton M  Zschack P  Hong H  Chiang T-C
Institution:X-ray Imaging Group, Center for Nanoscale Materials, Argonne National Laboratory, Argonne, Illinois 60439, USA.
Abstract:We report a study of critical x-ray scattering from SrTiO3 near the antiferrodistortive structural phase transition at T(C) approximately 105 K. A line shape analysis of the thermal diffuse scattering results in the most precise experimental determination to date of the critical exponent gamma. The microscopic mechanism behind the anomalous "central peak" critical scattering component is clarified here by the first-ever observation of a static coherent diffraction pattern (speckle pattern) within the anomalous critical scattering of SrTiO3. This observation allows us to directly attribute the origins of the central peak to Bragg diffraction from remnant static disorder above T(C).
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