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Direct-comb molecular spectroscopy with accurate, resolved comb teeth over 43 THz
Authors:Zolot A M  Giorgetta F R  Baumann E  Nicholson J W  Swann W C  Coddington I  Newbury N R
Institution:National Institute of Standards and Technology, Boulder, Colorado 80305, USA. Alex.Zolot@nist.gov
Abstract:We demonstrate a dual-comb spectrometer using stabilized frequency combs spanning 177 to 220 THz (1360 to 1690 nm) in the near infrared. Comb-tooth-resolved measurements of amplitude and phase generate over 4×10(5) individually resolved spectral elements at 100 MHz point spacing and kilohertz-level resolution and accuracy. The signal-to-noise ratio is 100 to 3000 per comb tooth. Doppler-broadened phase and amplitude spectra of CO(2), CH(4), C(2)H(2), and H(2)O in a 30 m multipass cell agree with established spectral parameters, achieving high-resolution measurements with optical bandwidth generally associated with blackbody sources.
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