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Magnetic Interactions in Insulating BEDT-TTF Salts
Authors:Takehiko Mori
Institution:Department of Organic and Polymeric Materials, Tokyo Institute of Technology, O-okayama, Meguro-ku, Tokyo, 152-8552, Japan
Abstract:Inter-dimer magnetic interactions J in BEDT-TTF (bis(ethylenedithio)tetrathiafulvalene) salts in the Mott insulator regime are estimated from the intermolecular overlap integrals. The estimated J values are compared with the experimental results, and the stable spin alignment and the dimensionality of the spin systems are discussed.
Keywords:charge transfer salts  πd-interaction  Mott insulator  molecule-based magnetism  
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