Calibrated U-TH glasses for neutron dosimetry and determination of uranium and thorium concentration by the fission track method |
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Authors: | J. W. H. Schreurs A. M. Friedman D. J. Rokop M. W. Hair R. M. Walker |
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Affiliation: | 1. Corning Glass Works , Corning, New York, 14830;2. Argonne National Laboratory , Argonne, Illinois, 60440;3. Washington University , St. Louis, Missouri, 63130 |
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Abstract: | We have prepared a series of standard uranium glasses. A primary standard containing 41 ppm of added U had its concentration and isotope ratio verified by mass spectrometry and by fission track techniques. Secondary standards were compared to the primary standard using the fission track technique. These glasses are useful for measuring both Th and U in solids. The U concentration in an unknown is determined by comparing the fission track density induced by thermal neutron irradiation with the corresponding density in the standard. Th is measured by a cyclotron irradiation using the same U standards. The glasses are also useful for neutron dosimetry. Investigators may obtain small samples of most of these standards from R. H. Brill of the Corning Museum of Glass. Although most of the glasses were fabricated from depleted uranium, one standard containing natural uranium is available. A standard Th glass with concentration of 41 ppm was also made. |
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Keywords: | Scintillator efficiency CeF3 Band structure calculations DFT FP-LMTO |
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