Structure and melting of dipole clusters |
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Authors: | Yu E Lozovik E A Rakoch |
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Institution: | (1) Institute of Spectroscopy, Russian Academy of Sciences, 142092 Troitsk, Moscow District, Russia |
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Abstract: | Two-dimensional microclusters made up of particles repelled by the dipole law and confined by an external quadratic potential
are considered. The model describes a number of physical systems, in particular, electrons in semiconductor structures near
a metallic electrode, indirect excitons in coupled semiconductor dots etc. Two competing types of particle ordering in clusters
have been revealed: formation of a triangular lattice and of a shell structure. Equilibrium configurations of clusters with
N=1–40 particles are calculated. Temperature dependences of the structure, potential energy, and mean-square radial and angular
displacements are studied. These characteristics are used to investigate cluster melting. Melting occurs in one or two stages,
depending on N. Melting of a two-shell microcluster takes place in two stages: at low temperatures—from the frozen phase to a state with
rotationally reoriented “crystalline” shells with respect to one another, followed by a transition involving breakdown of
radial order. Melting in a cluster made up of a larger number of shells occurs in one stage. This is due to the fact that
the potential barrier to intershell rotation is substantially lower than that to particle jumping from one shell to another
for small N, and of the same order of magnitude for large N. A method is proposed for predicting the character of melting in shell clusters by comparing the potential barriers for shell
rotation and intershell particle jumping.
Fiz. Tverd. Tela (St. Petersburg) 40, 1379–1386 (July 1998) |
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