Copper-based metal-organic frameworks for electrochemical reduction of CO2 |
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Affiliation: | 1. Shenzhen Key Laboratory of Polymer Science and Technology, Guangdong Research Center for Interfacial Engineering of Functional Materials, College of Materials Science and Engineering, Shenzhen University, Shenzhen 518060, China;2. School of Mechanical Engineering, University of South China, Hengyang 421001, China;1. School of Biomedical Engineering, Sun Yat-sen University, Shenzhen 518107, China;2. Department of Cardiology, The Affiliated TCM Hospital of Guangzhou Medical University, Guangzhou 510120, China;3. Bioscience and Biomedical Engineering Thrust, The Hong Kong University of Science and Technology (Guangzhou), Guangzhou 511400, China;4. Division of Life Science, Hong Kong University of Science and Technology, Hong Kong 999077, China;1. Key Laboratory of Aerosol Chemistry and Physics, State Key Laboratory of Loess and Quaternary Geology (SKLLQG), Institute of Earth Environment, Chinese Academy of Sciences, Xi''an 710061, China;2. Center of Excellence in Quaternary Science and Global Change, Chinese Academy of Sciences, Xi''an 710061, China;3. University of Chinese Academy of Sciences, Beijing 100049, China;4. Department of Environmental Science and Engineering, Xi''an Jiaotong University, Xi''an 710049, China;1. School of Materials Science and Engineering, Jiangsu Province Engineering Research Center of Intelligent Manufacturing Technology for the New Energy Vehicle Power Battery, Changzhou University, Changzhou 213164, China;2. School of Physics and Electronics, Hunan University, Changsha 410082, China;3. College of Chemistry and Materials Engineering, Hunan University of Arts and Science, Changde 415000, China;4. School of Chemistry, Tiangong University, Tianjin 300387, China;1. School of Chemistry and Chemical Engineering, Jiangsu University, Zhenjiang 212013, China;2. School of Resource and Environmental Engineering, Jilin Institute of Chemical Technology, Jilin 132000, China;1. Key Laboratory of Poyang Lake Environment and Resource Utilization of Ministry of Education, School of Resources & Environment, Nanchang University, Nanchang 330031, China;2. Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle, Nanchang Hangkong University, Nanchang 330063, China;3. School of Chemistry & Molecular Engineering, East China University of Science and Technology, Shanghai 200237, China |
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Abstract: | The electrochemical CO2 reduction reaction (CO2ER) is an emerging process that involves utilizing CO2 to produce valuable chemicals and fuels by consuming excess electricity from renewable sources. Recently, Cu and Cu-based nanoparticles, as earth-abundant and economical metal sources, have been attracting significant interest. The chemical and physical properties of Cu-based nanoparticles are modified by different strategies, and CO2 can be converted into multicarbon products. Among various Cu-based nanoparticles, Cu-based metal-organic frameworks (MOFs) are gaining increasing interest in the field of catalysis because of their textural, topological, and electrocatalytic properties. In this minireview, we summarized and highlighted the main achievements in the research on Cu-based MOFs and their advantages in the CO2ER as electrocatalysts, supports, or precursors. |
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