Investigation on third-order nonlinear optical properties of two Au(dmit)2/PMMA thin films by Z-scan technique in picosecond pulse regime |
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Authors: | Heliang Fan Xinqiang Wang Quan Ren Tingbin Li Dong Xu |
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Affiliation: | 1. School of Material Science and Engineering, China University of Mining and Technology, Xuzhou, China 2. State Key Laboratory of Crystal Materials and Institute of Crystal Materials, Shandong University, Jinan, 250100, China 3. Department of Optics, Shandong University, Jinan, 250100, China 4. Department of Materials and Chemical Engineering, Taishan University, Taian, 271021, China
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Abstract: | The third-order nonlinear optical properties of two Au(dmit)2/PMMA compound thin films, hexadecyltrimethylammonium bis(1,3-dithiole-2-thione-4,5-dithiolato)aurate and tetramethylammonium bis(1,3-dithiole-2-thione-4,5-dithiolato)aurate (abbreviated as MeAu and CtAu, respectively) with a doping concentration of 1?wt.% deposited on quartz-glass substrate were characterized by a single beam Z-scan technique at 1064?nm with 20?ps laser pulse width and 10?Hz repetition rate. The dominant nonlinear refraction and tiny nonlinear absorption of both materials lead to a larger possibility for them to be applied as promising candidates of all-optical switching. The results of two figures of merit, |W|?1 and |T|?1, were also calculated; this further validated the excellent properties of the materials for applications of the nonlinear optics. |
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