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On non-exponential unimolecular dissociation of molecules prepared by vibrational overtone excitation |
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| Affiliation: | 1. Qingdao Agricultural University, Department of Chemistry and Pharmacy, China;1. School of Mathematics, Renmin University of China, Beijing, China;2. Yau Mathematical Sciences Center, Tsinghua University, Beijing, China;3. Department of Mathematics, Harvard University, Cambridge, MA, USA |
| Abstract: | The sensitivity of vibrational overtone excitation experiments to non-RRKM behavior is considered. It is proposed that the experimental results are not inconsistent with intrinsically non-RRKM unimolecular lifetime distribution. |
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