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Method for analytical calculation of the nonlinear optical properties of polyatomic molecules in the MO LCAO approximation
Authors:K. M. Grushetskii
Abstract:Analytical expressions are obtained for any orders of the polarizabilities of polyatomic molecules as functions of the dipole integrals and derivatives of the matrix for the orders of the bonds over the field components. A procedure for calculating these polarizabilities is suggested. Belorussian State University of Information Science and Radioelectronics, 6, P. Brovka St., Minsk, 220600, Belarus. Translated from Zhurnal Prikladnoi Spektroskopii, Vol. 65, No. 3, pp. 436–438, May–June, 1998.
Keywords:spectrum  polarizability  molecular orbitals
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