Current-induced embrittlement of atomic wires |
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Authors: | Todorov T N Hoekstra J Sutton A P |
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Affiliation: | School of Mathematics and Physics, The Queen's University of Belfast, Belfast BT7 1NN, United Kingdom. T.Todorov@qub.ac.uk |
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Abstract: | Recent experiments suggest that gold single-atom contacts and atomic chains break at applied voltages of 1 to 2 V. In order to understand why current flow affects these defect-free conductors, we have calculated the current-induced forces on atoms in a Au chain between two Au electrodes. These forces are not by themselves sufficient to rupture the chain. However, the current reduces the work to break the chain, which results in a dramatic increase in the probability of thermally activated spontaneous fracture of the chain. This current-induced embrittlement poses a fundamental limit to the current-carrying capacity of atomic wires. |
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