Multi-mode absorption spectroscopy, MUMAS, using wavelength modulation and cavity enhancement techniques |
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| Authors: | M L Hamilton G A D Ritchie Y Arita P Ewart |
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| Institution: | 1. Department of Chemistry, The Physical and Theoretical Chemistry Laboratory, University of Oxford, South Parks Road, Oxford, OX1 3QZ, UK
2. Physics Department, Clarendon Laboratory, University of Oxford, Parks Road, Oxford, OX1 3PU, UK
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| Abstract: | Multi-mode absorption spectroscopy, MUMAS, has been combined with the techniques of wavelength modulation spectroscopy, WMS, and cavity enhanced absorption spectroscopy, CEAS, to record multiple molecular transitions using a single laser and a single detector. MUMAS signals were recorded using a multi-mode diode laser of the A-band $b^{1}\varSigma _{g}^{+}\leftarrow X^{3}\varSigma _{g}^{-}Multi-mode absorption spectroscopy, MUMAS, has been combined with the techniques of wavelength modulation spectroscopy, WMS,
and cavity enhanced absorption spectroscopy, CEAS, to record multiple molecular transitions using a single laser and a single
detector. MUMAS signals were recorded using a multi-mode diode laser of the A-band
b1\varSigma g+? X3\varSigma g-b^{1}\varSigma _{g}^{+}\leftarrow X^{3}\varSigma _{g}^{-} of molecular oxygen at 760 nm. Direct MUMAS and WMS-MUMAS signals were recorded using a White cell for air and pure oxygen
for pressures in the range 0 to 1 bar. CEAS-MUMAS signals were recorded with and without WMS in an open enhancement cavity
containing laboratory air. Enhancement of the signal-to-noise ratio has been obtained demonstrating the potential for increased
detection sensitivity for gas-sensing applications of MUMAS. |
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