| Conversion of Methane to C2 Hydrocarbons via Cold Plasma Reaction |
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| 引用本文： | BaoweiWang GenhuiXu. Conversion of Methane to C2 Hydrocarbons via Cold Plasma Reaction[J]. 天然气化学杂志, 2003, 12(3): 178-182 |
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| 作者姓名： | BaoweiWang GenhuiXu |
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| 作者单位： | SchoolofChemicalEngineeringandTechnology,TianjinUniversity,Tianjin300072,China |
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| 摘 要： | Direct conversion of methane to C2 hydrocarbons via cold plasma reaction with catalysts has been studied at room temperature and atmospheric pressure. Methane can be converted into C2 hydrocarbons in different selectivity depending on the form of the reactor, power of plasma, flow rate of methane, ratio of N2/CH4 and nature of the catalysts. The selectivity to C2 hydrocarbons can reach as high as 98.64%, and the conversion of methane as high as 60% and the yield of C2 hydrocarbons as high as 50% are obtained. Coking can be minimized under the conditions of: proper selection of the catalysts, appropriate high flow rate of inlet methane and suitable ratio of N2 to CH4. The catalyst surface provides active sites for radical recombination.
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| 关 键 词： | 甲烷 C2烃 低温等离子体 催化剂 天然气 制备 |
Conversion of Methane to C2 Hydrocarbons via Cold Plasma Reaction |
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| Baowei Wang,Genhui Xu. Conversion of Methane to C2 Hydrocarbons via Cold Plasma Reaction[J]. Journal of Natural Gas Chemistry, 2003, 12(3): 178-182 |
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| Authors: | Baowei Wang Genhui Xu |
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| Affiliation: | School of Chemical Engineering and Technology, Tianjin University, Tianjin 300072, China |
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| Abstract: | Direct conversion of methane to C2 hydrocarbons via cold plasma reaction with catalysts has been studied at room temperature and atmospheric pressure. Methane can be converted into C2 hydrocarbons in different selectivity depending on the form of the reactor, power of plasma, flow rate of methane, ratio of N2/CH4 and nature of the catalysts. The selectivity to C2 hydrocarbons can reach as high as 98.64%, and the conversion of methane as high as 60% and the yield of C2 hydrocarbons as high as 50% are obtained. Coking can be minimized under the conditions of: proper selection of the catalysts, appropriate high flow rate of inlet methane and suitable ratio of N2 to CH4. The catalyst surface provides active sites for radical recombination. |
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| Keywords: | methane C_2 hydrocarbons cold plasma catalyst |
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