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Construction of the azocane (azacyclooctane) moiety of the Lycopodium alkaloid lycopladine H via an intramolecular hydroaminomethylation strategy
Authors:Sacher Joshua R  Weinreb Steven M
Institution:Department of Chemistry, The Pennsylvania State University, University Park, Pennsylvania 16802, USA.
Abstract:An efficient synthetic strategy has been developed for annulation of an azocane ring onto a bicyclo2.2.2]octane scaffold via an intramolecular hydroaminomethylation protocol to generate an advanced intermediate bearing three of the four rings of the structurally unique Lycopodium alkaloid lycopladine H (1).
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