Interaction of a low-pressure gas flame and heterogeneous catalytic processes on the reactor surface |
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Authors: | E. N. Aleksandrov S. N. Kozlov N. M. Kuznetsov |
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Affiliation: | (1) Emanuel Institute of Biochemical Physics, Russian Academy of Sciences, ul. Kosygina 4, Moscow, 119991, Russia |
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Abstract: | Conclusions (1) It was shown that the Semenov theory in various modes of chain termination quantitatively describes oxyhydrogen combustion near the first ignition limit with allowance for the interaction between the flame and the catalytic processes on the reactor wall. (2) Numerical modeling of oxyhydrogen ignition in the diffusion-controlled chain-termination mode detected the dependence of the rate “constant” for heterogeneous chain initiation on the model of the reaction in the gas. (3) For the first time, the change in the specific rate of heterogeneous chain initiation during a single ignition was determined. (4) method for controlling the low-pressure flame mode by affecting tubes far from the reactor was proposed and applied. Original Russian Text ? E.N. Aleksandrov, S.N. Kozlov, N.M. Kuznetsov, 2006, published in Doklady Akademii Nauk, 2006, Vol. 407, No. 5, pp. 630–633. Presented by Academician A.E. Shilov October 5, 2005 |
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