Development of efficient photocatalytic systems for CO2 reduction using mononuclear and multinuclear metal complexes based on mechanistic studies |
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| Authors: | Hiroyuki Takeda Osamu Ishitani |
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| Institution: | 1. Toyota Central R&D Labs., Inc., 41-1 Yokomichi, Nagakute, Aichi 480-1192, Japan;2. CREST/JST, Japan;3. Department of Chemistry, Graduate School of Science and Engineering, Tokyo Institute of Technology, 2-12-1-E1-9 O-okayama, Meguro-ku, Tokyo 152-8551, Japan;4. SORST/JST and CREST/JST, Japan |
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| Abstract: | Photocatalytic systems for CO2 reduction using metal complexes, especially rhenium(I) complexes as a main component, are reviewed: mononuclear Re(I) complexes, mixed systems with two different Re(I) complexes, and supramolecule systems with a Re(I) complex connected to a ruthenium(II) complex. We focus on the mechanistic studies and the architecture for constructing the photocatalytic systems based on the mechanism. |
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