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JRQ and JPA irradiated and annealed reactor pressure vessel steels studied by positron annihilation
Authors:Vladimír Slugeň  Oleksandr Gokhman  Stanislav Pecko  Stanislav Sojak  Frank Bergner
Institution:1. Institute of Nuclear and Physical Engineering, Slovak University of Technology, Ilkovi?ova 3, 81219 Bratislava, Slovakiavladimir.slugen@stuba.sk;3. Institute of Nuclear and Physical Engineering, Slovak University of Technology, Ilkovi?ova 3, 81219 Bratislava, Slovakia;4. Institute of Physics and Mathematics, South Ukrainian National Pedagogical University, Staroportofrankovkaya 26, 65020 Odesa, Ukraine;5. Helmholtz-Zentrum Dresden-Rossendorf, Institute of Ion Beam Physics and Materials Research, Bautzner Landstr. 400, 01328 Dresden, Germany
Abstract:The paper is focused on a comprehensive study of JRQ and JPA reactor pressure vessel steels from the positron annihilation lifetime spectroscopy (PALS) point of view. Based on our more than 20 years’ experience with characterization of irradiated reactor steels, we confirmed that defects after irradiation start to grow and/or merge into bigger clusters. Experimental results shown that JPA steel is more sensitive to the creation of irradiation-induced defects than JRQ steel. It is most probably due to high copper content (0.29?wt.% in JPA) and copper precipitation has a major impact on neutron-induced defect creation at the beginning of the irradiation. Based on current PALS results, no large vacancy clusters were formed during irradiation, which could cause dangerous embrittlement concerning operation safety of nuclear power plant. The combined PALS, small angle neutron scattering and atomic probe tomography studies support the model for JRQ and JPA steels describing the structure of irradiation-induced clusters as agglomerations of vacancy clusters (consisting of 2–6 vacancies each) and are separated from each other by a distribution of atoms.
Keywords:Nuclear materials  positron annihilation spectroscopy  RPV steel  irradiation  ion beam implantation
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