Quantum criticality in an organic magnet |
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Authors: | Stone M B Broholm C Reich D H Tchernyshyov O Vorderwisch P Harrison N |
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Institution: | Condensed Matter Sciences Division, Oak Ridge National Laboratory, Oak Ridge, Tennennesse 37831, USA. |
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Abstract: | Exchange interactions between S=1/2 sites in piperazinium hexachlorodicuprate produce a frustrated bilayer magnet with a singlet ground state. We have determined the field-temperature phase diagram by high field magnetization and neutron scattering experiments. There are two quantum critical points: Hc1=7.5 T separates a quantum paramagnet phase from a three dimensional, antiferromagnetically ordered state while Hc2=37 marks the onset of a fully polarized state. The ordered phase, which we describe as a magnon Bose-Einstein condensate (BEC), is embedded in a quantum critical regime with short range correlations. A low temperature anomaly in the BEC phase boundary indicates that additional low energy features of the material become important near Hc1. |
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