Analytical control of molecular excitations including strong field polarization effects |
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Authors: | Zou Shiyang Ren Qinghua Balint-Kurti Gabriel G Manby Frederick R |
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Affiliation: | School of Chemistry, University of Bristol, Bristol BS8 1TS, United Kingdom. |
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Abstract: | An analytical scheme is presented for designing a laser pulse to excite H2 from one specified vibrational-rotational state to another. The scheme is based on an adiabatic two-state approximation in a Floquet picture. By continuously and smoothly changing the laser frequency, we explicitly harness the dynamic Stark shifts and maintain resonance between the dressed diabatic states during laser-molecule interaction. The explicit time-dependent solution of the Schr?dinger equation confirms the validity and efficacy of the analytically designed laser pulses. The scheme depends on the molecular polarizability to achieve its control objectives. |
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