Self-Assembled Bilayers on Indium-Tin Oxide (SAB-ITO) Electrodes: A Design for Chromophore-Catalyst Photoanodes |
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| Authors: | Christopher R K Glasson Wenjing Song Dennis L Ashford Aaron Vannucci Zuofeng Chen Javier J Concepcion Patrick L Holland Thomas J Meyer |
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| Affiliation: | Department of Chemistry, University of North Carolina , Chapel Hill, North Carolina 27599-3290, United States. |
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| Abstract: | A novel approach for creating assemblies on metal oxide surfaces via the addition of a catalyst overlayer on a chomophore monolayer derivatized surface is described. It is based on the sequential self-assembly of a chromophore, [Ru(bpy)(4,4'-(PO(3)H(2)bpy)(2))](2+), and oxidation catalyst, [Ru(bpy)(P(2)Mebim(2)py)OH(2)](2+), pair, resulting in a spatially separated chromophore-catalyst assembly. |
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