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Transmutation studies using SSNTD and radiochemistry and the associated production of secondary neutrons
Authors:R. Brandt   M. Ochs   J. -S. Wan   Th. Schmidt   E. -J. Langrock   P. Vater   J. Adam   V. P. Bamblevskij   V. Bradnova   L. K. Gelovani   V. K. Kalinnikov   M. I. Krivopustov   B. A. Kulakov   A. N. Sosnin   V. P. Perelygin   V. S. Pronskikh   V. I. Stegailov   V. M. Tsoupko-Sitnikov   G. Modolo   R. Odoj   P. -W. Phiippen   J. -C. Adloff   F. Pape   M. Debeauvais   M. Zamani-Valassiadou   S. R. Hashemi-Nezhad   K. K. Dwivedi   S. -L. Guo   L. Li   Y. -L. Wang  B. Wilson
Affiliation:

a Kernchemie, FB 15, Philipps-University, D-35032, Marburg, Germany

b Joint Institute for Nuclear Research, Dubna 141980, Russia

c Forschungszentrum Jülich, FZJ, D-54245, Jülich, Germany

d Institute de Recherche Subatomique, University L. Pasteur, F-67037, Strasbourg, France

e Physics Department, Aristotle University, Thessaloniki 54006, Greece

f Falkiner High Energy Physics Dpt., University of Sydney, Sydney, NSW 2006, Australia

g Department of Chemistry, North-Eastern Hill University, Shillong 793003, India

h China Institute of Atomic Energy, Beijing 102413, China

i Los Alamos National Laboratory, Los Alamos, NM 87545, USA

Abstract:Experiments using 1.5 GeV, 3.7 GeV and 7.4 GeV protons from the Synchrophasotron, LHE, JINR, Dubna, Russia, on extended Pb- and U-targets were carried out using SSNTD and radiochemical sensors for the study of secondary neutron fluences. We also carried out first transmulation studies on the long-lived radwaste nuclei 129I and 237Np.

In addition, we carried out computer code simulation studies on these systems using LAHET and DCM/CEM codes. We have difficulties to understand rather large transmutation rates observed experimentally when they are compared with computer simulations. There seems to be a rather fundamental problem understanding the large transmutation rates as observed experimentally in Dubna and CERN, as compared to those theoretical computer simulations mentioned above.

Keywords:Transmutation   129I   237Np   enhanced nuclear cross-section
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