Speciation of239U and238Np produced by radiative neutron capture |
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Authors: | M Kadri J J Schleiffer J P Adloff |
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Institution: | (1) Centre de Recherches Nucléaires, Laboratoire de Chimie Nucléaire, BP 20, 67037 Strasbourg Cedex, France |
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Abstract: | Various simple and complex compounds of238U and237Np have been irradiated in a neutron flux. The chemical state of239U and238Np formed in (n, ) reactions has been determined as a function of the initial oxidation state of the actinide elements and of the nature of ligands. A scheme for the chemical reactions following neutron capture is proposed. |
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