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Field- and thickness-dependent performance of tandem organic light-emitting diodes with buffer-modified fullerene/copper phthalocyanine heterojunction as interconnector
Authors:Zhaoyue Lü  ,Xiong Li,Yue Wang,Jing Xiao,Penglai Xu
Affiliation:1. Department of Physics, School of Science, East China University of Science & Technology, Shanghai 200237, China;2. School of Science, Beijing Technology and Business University, Beijing 100048, China;3. Key Laboratory of Luminescence and Optical Information, Ministry of Education, Institute of Optoelectronic Technology, Beijing Jiaotong University, Beijing 100044, China;4. Physics and Electronic Engineering College, Taishan University, Shandong Province 271021, China
Abstract:Tandem organic light-emitting diodes (OLEDs) with the buffer-modified fullerene/copper phthalocyanine (LiF/C60/CuPc/MoO3) as interconnector have been investigated. The properties of tandem OLEDs are dependent on electric field, which is induced by electric-field-dependence of charge generation (by electric filed and photons) and separation in such an interconnector structure. At low electric field, because of less generated-charges and light-absorption of C60/CuPc film, current efficiency and brightness of tandem OLEDs with two emissive units exhibit less than twice higher than those of conventional single-unit device. But more than twofold enhancement of current efficiency and brightness is observed at higher electric field due to a large number of charges generated in the interconnector. Meanwhile, the performance of tandem devices is affected by the thickness of C60 and CuPc. The optimal thickness is related to their exciton diffusion length.
Keywords:Organic heterojunction   Electric-generated-charge   Photo-generated-charge   Fullerene   Copper phthalocyanine
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