Inclusion of discrete-to-continuum coupling in multiphoton excitation and dissociation calculations

A nonperturbative approach to multiphoton excitation and dissociation of molecules is presented in which coupling to the continuum is treated explicitly. Transitions among continuum levels are not modeled directly, but something of their effect is represented by assuming that the continuum population density is so low as to be effectively zero at all times. Two trial applications are briefly discussed.