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Electron dynamics triggered by double attosecond pulses: Simulations based on time-dependent density functional theory
Authors:Yalong Jiao  Feng Wang  Xuhai Hong  Wenyong Su  Zhen Zhang
Institution:1. School of Physics, Key Laboratory of Cluster Science of Ministry of Education, Beijing Institute of Technology, Beijing 100081, China;2. Laser Micro/Nano Fabrication Laboratory, School of Mechanical Engineering, Beijing Institute of Technology, Beijing 100081, China;3. School of Software, Beijing Institute of Technology, Beijing 100081, China
Abstract:In order to observe the high-field effect, the external laser field must reach its peak intensity before the electron ionization. To this end, it is important to reduce pulse duration to typical attosecond timescale. In this paper, the interaction electron dynamics between attosecond pulses and dielectric is investigated within the time-dependent density functional theory. Taking the CaF2 crystal as an example, we give a comparison of electron dynamics response between single and double pulses. Moreover, the nonlinear energy absorption and electron excitation processes are simulated by adjusting the polarization direction of the sub-pulse. Present results demonstrate that the double pulses show lower electron excitation and energy absorption than the single pulse, which is in accordance with experimental higher ablation threshold and smaller heat-affected zones of the double pulses. In addition, the curves of final excited electron number and energy absorption exhibit the quasi-symmetry about the axis of 180°, which has not been reported yet.
Keywords:Time-dependent density functional theory  Electron dynamics  Attosecond pulse  Polarization angle
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