Light-mediated heterogeneous cross dehydrogenative coupling reactions: metal oxides as efficient, recyclable, photoredox catalysts in C-C bond-forming reactions |
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| Authors: | Rueping Magnus Zoller Jochen Fabry David C Poscharny Konstantin Koenigs René M Weirich Thomas E Mayer Joachim |
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| Institution: | Institute of Organic Chemistry, RWTH Aachen University, Landoltweg 1, 52074 Aachen, Germany. magnus.rueping@rwth-aachen.de |
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| Abstract: | Let there be light: A heterogeneous photocatalytic system based on easily recyclable TiO(2) or ZnO allows cross dehydrogenative coupling reactions of tertiary amines. The newly developed protocols have successfully been applied to various C-C and C-P bond-forming reactions to provide nitro amines as well as amino ketones, nitriles and phosphonates. |
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