Thermal conductivity degradation induced by heavy ion irradiation at
room temperature in ceramic materials |
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Authors: | S Gomès L David J-P Roger G Carlot D Fournier C Valot M Raynaud |
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Institution: | (1) Centre de Thermique de Lyon, UMR CNRS 5008, CETHIL, INSA-Lyon, Batiment Sadi Carnot, 19 rue de la Physique, 69621 Villeurbanne Cedex, France;(2) Laboratoire d'Optique Physique, UPR A0005, ESPCI, 10 rue Vauquelin, 75005 Paris, France;(3) Unité DEC/SESC/Laboratoire des Lois de Comportement du Combustible, Batiment 315, CEA-Cadarache, 13108 Saint Paul lez Durance, France |
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Abstract: | The thermal conductivity degradation induced by irradiation with energetic heavy ions at room temperature is studied and quantified.
Three
semi-metallic systems: titanium and zirconium carbides, titanium nitride,
as well as a covalent compound: 6H silicon carbide were irradiated by 25.8 MeV krypton ions at 1016 and 6 . 1016 ions.cm-2 doses to
produce defects. During ion irradiation, inelastic collisions and elastic
collisions occur at a different depth in a material. Two collision domains
can be defined. Modulated thermoreflectance microscopy measurements were
performed at differing frequencies to characterize the thermal conductivity
degradation in these two domains for each of the investigated materials. Our
results reveal a significant thermal conductivity degradation in the two
collision domains for all materials. Elastic collisions are shown to degrade
more strongly the thermal properties than inelastic ones. Scattering of
thermal energy carriers is larger in elastic collision domain because
displacement cascades produce a very high concentration of point defects:
vacancies, interstitials and implanted Kr ions. The degradation coming from
electronic interactions that seems to be more important in SiC can be
explained by the presence of large populations of generated extended
defects, facing to generated individual point defects in TiC, TiN or ZrC. |
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