Dissociation dynamics of Ar3 in the time-dependent self-consistent field (TDSCF) approximation |
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| Authors: | V Buch RB Gerber MA Ratner |
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| Institution: | Department of Physical Chemistry and Fritz Haber Research Center for Molecular Dynamics, The Hebrew University of Jerusalem, Jerusalem 91904, Israel;Department of Chemistry, Northwestern University, Evanston, Illinois 60201, USA |
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| Abstract: | The TDSCF approximation is applied to dissociation of Ar3, which exhibits strong-coupling behavior (efficient internal energy transfer). The TDSCF results are in excellent agreement with those of exact classical dynamics. Combined with earlier findings for weak-coupling cases, this suggests validity of TDSCF for dissociation at all coupling strengths. |
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