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Magnetic properties of RCr2Si2 compounds (R=Tb,Er)
Authors:Marcela Janatová  Jana Poltierová Vejpravová  Martin Divi?
Affiliation:1. Key Laboratory of Cryogenics, Technical Institute of Physics and Chemistry, Chinese Academy of Sciences, Beijing, China;2. School of Material Science and Engineering, Hebei University of Technology, Tianjin, China;3. State Key Laboratory of Magnetism, Beijing National Laboratory for Condensed Matter, Physics and Institute of Physics, Chinese Academy of Sciences, Beijing, China;1. State Key Laboratory of Advanced Special Steels & Shanghai Key Laboratory of Advanced Ferrometallurgy & School of Materials Science and Engineering, Shanghai University, Shanghai 200072, China;2. Institute of Materials Physics, University of Münster, Wilhelm-Klemm-Straße 10, D-48149 Münster, Germany;3. Beijing Key Laboratory of Biomass Waste Resource Utilization, Biochemical Engineering College, Beijing Union University, Beijing 100023, China;1. Department of Physics, Nanjing University of Information Science & Technology, Nanjing 210044, China;2. Department of Physics, Nanjing Normal University, Nanjing 210097, China;1. Innovative Center for Advanced Materials (ICAM), Hangzhou Dianzi University, Hangzhou 310012, PR China;2. Key Laboratory of Electromagnetic Processing of Materials (Ministry of Education), Northeastern University, Shenyang 110819, PR China;3. Institut für Anorganische und Analytische Chemie, Universität Münster, D-48149 Münster, Germany
Abstract:We report on magnetic properties of RCr2Si2 compounds with R=Tb, Er. The polycrystalline samples were characterized by powder X-ray diffraction and found to be isostructurally crystallizing in the ThCr2Si2-type tetragonal structure. The samples were further investigated by specific heat, AC-susceptibility and magnetization methods in the temperature range 2–900 K and in magnetic fields up to 9 T. The magnetic measurements revealed the magnetic ordering of the rare-earth moments below about 2 K, whilst no high-temperature ordering of the Cr moments was observed. The evidence of for Cr magnetism is corroborated by results of first-principles calculations based on the density functional theory (DFT).
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