Magnetic and transport properties of Nd1.67Sr0.33NiO4 |
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Authors: | M Zaghrioui F GiovannelliS Pruvost N PoirotI Monot-Laffez |
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Institution: | Laboratoire d’Electrodynamique des Matériaux Avancés, UMR 6157 CNRS—CEA, Université François Rabelais, IUT de Blois, C.S. 2903, 3 place Jean Jaurès 41029 Blois cedex, France |
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Abstract: | Nd1.67Sr0.33NiO4 polycrystals have been prepared by modified sol–gel method and subsequent annealing. X-ray diffraction analysis, electrical resistivity, magnetic susceptibility and thermal magnetisation have been measured. Rietveld analyses show a tetragonal or pseudo-tetragonal K2NiF4-type structure. The resistivity measurements present a change in conduction mode close to 230 K, which corresponds to the charge ordering temperature. Below this temperature, the material adopts a variable range hopping conduction mode; and above, the conduction follows adiabatic thermal activated mode. The magnetic measurements show paramagnetic behaviour in the range of 80–300 K. Moreover, the magnetic susceptibility data show a sign of the charge ordering transition about 230 K. |
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Keywords: | Charge ordering Nickelates Resistivity Magnetic susceptibility |
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