Simultaneous operation at two different wavelengths of an PrLaP5O14 laser

Simultaneous laser operation at the wavelengths of λ₁=637 and λ₂=717 in Pr_0.5La_0.5P₅O₁₄ single crystals was observed. The crystals were excited by nanosecond publses from a Coumarin 2 dye laser (λ=450 nm). Laser emissions and their interdependence were studied both in crystals without an external resonator and in crystals placed within a plane parallel resonator. The energetic, time and frequency characteristics for both laser actions were examined. The effect of bifrequential emission was also found in crystals of different ratios of Pr and La ions concentration and in pure praseodymium pentaphosphate.