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Photoelectron spectroscopy of two-photon ionisation of rare-gas atoms by multiple high order harmonics
Authors:K. Furusawa  T. Okino  T. Shimizu  H. Hasegawa  Y. Nabekawa  K. Yamanouchi  K. Midorikawa
Affiliation:(1) Laser Technology Laboratory, RIKEN, 2-1, Hirosawa, Wako, Saitama 351-0198, Japan;(2) School of Science, University of Tokyo, Hongo, Bunkyo-ku, Tokyo 113-0033, Japan;(3) Institute for Molecular Science, Myodaiji, Okazaki 444-8585, Japan
Abstract:Two-photon ionisation processes of rare-gas atoms produced by a superposition of multiple high order harmonics are studied by using a photoelectron spectroscopy technique. Second-order nonlinearity is confirmed by comparing the intensity-dependent photoelectron yields between the linear and nonlinear processes, and the cross sections of these processes are estimated. We also demonstrate the autocorrelation measurement of harmonic envelopes as a preliminary step toward characterisation of an attosecond pulse train. PACS 32.80.Fb; 32.80.Wr; 42.65.-k
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