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被动多轴DOAS技术污染气体垂直柱浓度反演方法研究
引用本文:付强,刘文清,司福祺.被动多轴DOAS技术污染气体垂直柱浓度反演方法研究[J].光子学报,2009,38(5):1216-1220.
作者姓名:付强  刘文清  司福祺
作者单位:付强,FU Qiang(中国科学院安徽光学精密机械研究所,环境光学与技术重点实验室,合肥,230031;中国环境监测总站,北京,100029);刘文清,司福祺,张英华,谢品华,LIU Wen-qing,SI Fu-qi,ZHANG Ying-hua,XIE Pin-hua(中国科学院安徽光学精密机械研究所,环境光学与技术重点实验室,合肥,230031)  
基金项目:中国高技术研究和发展基金,中国科学院知识创新工程重大项目 
摘    要:介绍了基于太阳散射光的多轴被动差分吸收光谱技术与系统及其在大气污染气体垂直柱浓度监测中的应用.实验中利用夫琅和费光谱作为参考光谱,同时将Ring光谱作为一种吸收结构参与拟合去除太阳光谱中的夫琅和费结构和Ring效应对测量结果的影响,并结合辐射传输模型将污染气体斜柱浓度转换为垂直柱浓度,通过“好运北京”奥运限车期间与OMI卫星的对比实验一致得出限车期间NO2有约20%的下降,证实了本方法的可行性.

关 键 词:被动差分吸收光谱技术  多轴  垂直柱浓度  Ring效应
收稿时间:2008-03-24
修稿时间:2008-05-07

Determination of the Vertical Column Density of Trace Gas Measured by MAX-DOAS
FU Qiang,LIU Wen-Qing,CI Fu-Qi,ZHANG Ying-Hua,XIE Pin-Hua.Determination of the Vertical Column Density of Trace Gas Measured by MAX-DOAS[J].Acta Photonica Sinica,2009,38(5):1216-1220.
Authors:FU Qiang  LIU Wen-Qing  CI Fu-Qi  ZHANG Ying-Hua  XIE Pin-Hua
Institution:(1 Key Laboratory of Environmental Optics |and |Technology|Anhui Institute of Optics and Fine Mechanics,
Chinese Academy of Sciences,Hefei 230031,China)
(2 Environmental monitoring of China,Beijing 100029,China)
Abstract:The method and system of determination of trace gas vertical column density by passive MAX-DOAS were described.A so called Fraunhofer spectrum was used as reference spectrum in the DOAS fitting process to reduce the influence of Fraunhofer lines.Ring spectrum was included in the DOAS fitting process as an additional absorber to decrease the Ring effect.And slant column density was converted into vertical column density by the radiative transfer model.Through compare with Dutch-Finnish nadir-pointing spectrometer (OMI) in the period of “Good Luck Beijing” Olympic test games,good correlation was proved.
Keywords:Passive differential optical absorption spectroscopy  Max axes  Vertical column density  Ring effect
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