Tunable amplified spontaneous emissions by dimensional-controlled microcrystal synthesis |
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Authors: | Hui-Ying Liu Ye-Fen Li Qing-Gang Gao Zhen-Dong Liu Hong-Bing Fu |
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Institution: | a School of Materials Science and Engineering, Beijing Institute of Fashion Technology, Beijing 100029, China;
b Beijing Key Laboratory for Optical Materials and Photonic Devices, Department of Chemistry, Capital Normal University, Beijing 100048, China |
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Abstract: | The excited-state intramolecular proton transfer molecules based on chalcone (E)-3-(4'-dimethylaminophenyl)-1-(4'-fluoro-2'-hydroxyphenyl)-2-propen-1-one (DMF-HPPO) have been synthesized under microwave irradiation. One-dimensional (1D) microwires and 2D microdisks of DMF-HPPO have been selectively prepared by controlling the solution polarity. XRD results revealed the two microcrystals exhibit distinct diffraction patterns, which indicates that they have belonged to different crystalline nature. The microcrystals demonstrate shape-dependent amplified spontaneous emissions (ASE) that the emission of 1D microwire is central around 618 nm and the 2D microdisk emits fluorescence at 650 nm. This result reveals the controlled synthesis of two microcrystals and their consequent multicolor amplified spontaneous emission, providing considerable promise for the development and application of new opto-electronic devices. |
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Keywords: | Amplified spontaneous emission Self-assembly Microstructures Luminescence Optical properties |
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