Field-induced spin-flip and spin-flip transitions in PrGa2

A detailed neutron diffraction study of a single crystal of hexagonal PrGa₂ under an applied field is presented. The field is applied along the easy 100] direction of the hexagonal plane. The compound exhibits several field-induced magnetic structures and, in particular, an uncompensated long period commensurate antiphase structure defined by the propagation vector (4/27, 4/27, 0) at zero field and below T_t = 3.5 K. Concerning the intermediate magnetic structures below T_t, two types of magnetic phase transitions are observed: a spin-flip transition where one moment per magnetic cell turns over, and a spin-slip transition from the low field commensurate propagation vector (4/27, 4/27, 0) to another commensurate vector (1/7, 1/7, 0). Between T_t and T_N = 7.2 K, the structure becomes apmlitude-modulated with a propagation vector (0.148, 0.148, 0.023). Important and original magnetic domain effects are also observed due to the high degeneracy of the easy direction of the hexagonal plane in both T<T_t and T_t<T<T_N regions.