Scalable Low‐Cost SnS2 Nanosheets as Counter Electrode Building Blocks for Dye‐Sensitized Solar Cells |
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Authors: | Yang Bai Dr Xu Zong Dr Hua Yu Dr Zhi‐Gang Chen Prof Lianzhou Wang |
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Institution: | 1. Nanomaterials Centre, School of Chemical Engineering and AIBN, The University of Queensland, Brisbane, QLD 4072 (Australia);2. Materials Engineering, The University of Queensland, Brisbane, QLD 4072 (Australia) |
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Abstract: | A new type of semitransparent SnS2 nanosheet (NS) films were synthesized using a simple and environmentally friendly solution‐processed approach, which were subsequently used as a counter electrode (CE) alternative to the noble metal Pt for triiodide reduction in dye‐sensitized solar cells (DSSCs). The resultant SnS2‐based CE with a thickness of about 300 nm exhibited excellent electrochemical catalytic activity for catalyzing the reduction of triiodide and demonstrated comparable power conversion efficiency of 7.64 % with that of expensive Pt‐based CE in DSSCs (7.71 %). When functionalized with a small amount of carbon nanoparticles, the SnS2 NS‐based CE showed even better performance of 8.06 % than Pt under the same conditions. Considering the facile fabrication method, optical transparency, low cost, and remarkable catalytic property, this study on SnS2 NSs may shed light on the large‐scale production of electrocatalytic electrode materials for low‐cost photovoltaic devices. |
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Keywords: | dye‐sensitized solar cells efficient counter electrode nanostructures photochemistry SnS2 nanosheets |
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