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First experiments on transmutation studies of129I and237Np using relativistic protons of 3.7 GeV
Authors:M. I. Krivopustov  J. Adam  V. Bradnova  R. Brandt  V. S. Butsev  P. I. Golubev  V. G. Kalinnikov  J. Karachuk  B. A. Kulakov  E.-J. Langrock  G. Modolo  M. Ochs  R. Odoj  A. N. Premyshev  V. S. Pronskich  Th. Schmidt  V. I. Stegailov  J. S. Wan  V. M. Zupko-Sitnikov
Affiliation:(1) Joint Institute for Nuclear Research, JINR, Dubna, Russia;(2) Kernchemie, Philipps-Universität, Marburg, Germany;(3) Forschungszenstrum Jülich, FZJ, Jülich, Germany;(4) Northwest Institute of Nuclear Technology, Xian, P. R. China
Abstract:First experiments on the transmutation of long-lived129I and237Np using relativistic protons of 3.7 GeV are described. Relativistic protons generate in extended Pb-targets substancial neutron fluences. These neutrons get moderated in paraffin and are used for transmutation as follows:129I(n,gamma)130Ibetararr and237Np(n,gamma)238Npbetararr. The isotopes130I (T1/2-12.36 h) and238Np (T1/2=2.117 d) were identified radiochemically. One can estimate the transmutation cross-section (n,gamma) in the given neutron field as sgr(129I(n,gamma))=(10±2)b and sgr(237Np(n,gamma))=(140±30)b The experiments were carried out in November 1996 at the Synchrophasotron, LHE, Dubna, Russia. The investigation has been performed at the Laboratory of High Energies, JINR, Dubna.
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