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First experiments on transmutation studies of129I and237Np using relativistic protons of 3.7 GeV
Authors:M I Krivopustov  J Adam  V Bradnova  R Brandt  V S Butsev  P I Golubev  V G Kalinnikov  J Karachuk  B A Kulakov  E-J Langrock  G Modolo  M Ochs  R Odoj  A N Premyshev  V S Pronskich  Th Schmidt  V I Stegailov  J S Wan  V M Zupko-Sitnikov
Institution:(1) Joint Institute for Nuclear Research, JINR, Dubna, Russia;(2) Kernchemie, Philipps-Universität, Marburg, Germany;(3) Forschungszenstrum Jülich, FZJ, Jülich, Germany;(4) Northwest Institute of Nuclear Technology, Xian, P. R. China
Abstract:First experiments on the transmutation of long-lived129I and237Np using relativistic protons of 3.7 GeV are described. Relativistic protons generate in extended Pb-targets substancial neutron fluences. These neutrons get moderated in paraffin and are used for transmutation as follows:129I(n,gamma)130Ibetararr and237Np(n,gamma)238Npbetararr. The isotopes130I (T 1/2-12.36 h) and238Np (T 1/2=2.117 d) were identified radiochemically. One can estimate the transmutation cross-section (n,gamma) in the given neutron field as sgr(129I(n,gamma))=(10±2)b and sgr(237Np(n,gamma))=(140±30)b The experiments were carried out in November 1996 at the Synchrophasotron, LHE, Dubna, Russia. The investigation has been performed at the Laboratory of High Energies, JINR, Dubna.
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