Validity of the rotational sudden approximation for vibrational relaxation in He + CO |
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| Authors: | R.J. Price D.C. Clary G.D. Billing |
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| Affiliation: | Department of Chemistry, University of Manchester Institute of Science and Technology, Manchester M60 1QD, UK;Department of Chemistry, Panum Institute, DK-2200 Copenhagen, Denmark |
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| Abstract: | Calculations of cross sections and rate constants are reported for the vibrational relaxation of CO in collision with 3He and 4He. Results computed using a semiclassical technique and a vibrational close-coupling, rotational infinite-order sudden method are compared. |
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