Interet et obtention des courbes vitesse-degre d'avancement en cinetique heterogene |
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Authors: | G Thomas J J Gruffat M Soustelle |
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Institution: | (1) Laboratoire de Cinétique Hétérogène Département de Chimie, Ecole Nationale Supérieure des Mines, Saint-Etienne, France |
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Abstract: | Résumé Le plus souvent, l'étude de la cinétique d'une réaction hétérogène est faite en traÇant les courbes intégrales qui donnent les variations du degré d'avancement en fonction du temps. Depuis quelques années, on commence à utiliser les courbes vitesse-temps. Nous attirons l'attention sur l'importance des courbes vitesse-degré d'avancement, qui facilitent la mise en évidence des points singuliers, permettent l'étude de l'influence des facteurs extérieurs et peuvent rendre de grands services dans la recherche des mécanismes. Trois méthodes sont suggérées pour l'obtention de ces courbes, un exemple est donné pour la décomposition de l'hydrogénocarbonate de sodium.
The kinetics of heterogeneous reactions are in most cases studied by means of integral curves which represent the degree of reaction as a function of the time. Recently, rate vs. time curves have also been used for this purpose. The present paper draws attention to the importance of curves giving the degree of reaction as a function of the rate of reaction; these facilitate the investigation of separate points, make possible the interpretation of various factors, and provide valuable data concerning the mechanism. Three methods are suggested for preparing these curves and the decomposition of sodium hydrogen carbonate is given as an example.
Zusammenfassung Die Kinetik heterogener Reaktionen wird oft durch das Studium der durch die Darstellung der Änderungen des Fortschreitungsgrades als Funktion der Zeit erhaltenen Integralkurven untersucht. In neuester Zeit werden hierzu auch die Geschwindigkeits-Zeitkurven verwendet. Auf die Bedeutung der Kurven vom Fortschreitungsgrad als Funktion der Geschwindigkeit wird hingewiesen, diese erleichtern die Berücksichtigung einzelner Punkte. Weiterhin wurde die Untersuchung Äu\erer Faktoren ermöglicht und gute Ergebnisse bei der Prüfung des Mechanismus erhalten. Drei Methoden wurden zur Ermittlung dieser Kurven vorgeschlagen und ein Beispiel für die Zersetzung des Natriumbikarbonates gegeben.
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![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![lcy](/content/w81554m2m8760r62/xxlarge1083.gif) ![Acy](/content/w81554m2m8760r62/xxlarge1040.gif) ![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![Vcy](/content/w81554m2m8760r62/xxlarge1042.gif) ![Ocy](/content/w81554m2m8760r62/xxlarge1054.gif) ![Mcy](/content/w81554m2m8760r62/xxlarge1052.gif) ![Ocy](/content/w81554m2m8760r62/xxlarge1054.gif) ![zhcy](/content/w81554m2m8760r62/xxlarge1078.gif) ![Ncy](/content/w81554m2m8760r62/xxlarge1053.gif) ![ycy](/content/w81554m2m8760r62/xxlarge1099.gif) ![Icy](/content/w81554m2m8760r62/xxlarge1048.gif) ![scy](/content/w81554m2m8760r62/xxlarge1089.gif) ![scy](/content/w81554m2m8760r62/xxlarge1089.gif) ![lcy](/content/w81554m2m8760r62/xxlarge1083.gif) ![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![Dcy](/content/w81554m2m8760r62/xxlarge1044.gif) ![Ocy](/content/w81554m2m8760r62/xxlarge1054.gif) ![Vcy](/content/w81554m2m8760r62/xxlarge1042.gif) ![Acy](/content/w81554m2m8760r62/xxlarge1040.gif) ![Ncy](/content/w81554m2m8760r62/xxlarge1053.gif) ![Icy](/content/w81554m2m8760r62/xxlarge1048.gif) ![Rcy](/content/w81554m2m8760r62/xxlarge1056.gif) ![Acy](/content/w81554m2m8760r62/xxlarge1040.gif) ![zhcy](/content/w81554m2m8760r62/xxlarge1078.gif) ![lcy](/content/w81554m2m8760r62/xxlarge1083.gif) ![Icy](/content/w81554m2m8760r62/xxlarge1048.gif) ![Ncy](/content/w81554m2m8760r62/xxlarge1053.gif) ![ycy](/content/w81554m2m8760r62/xxlarge1099.gif) ![Fcy](/content/w81554m2m8760r62/xxlarge1060.gif) ![Acy](/content/w81554m2m8760r62/xxlarge1040.gif) ![kcy](/content/w81554m2m8760r62/xxlarge1082.gif) ![tcy](/content/w81554m2m8760r62/xxlarge1090.gif) ![Ocy](/content/w81554m2m8760r62/xxlarge1054.gif) ![Rcy](/content/w81554m2m8760r62/xxlarge1056.gif) ![Ocy](/content/w81554m2m8760r62/xxlarge1054.gif) ![Dcy](/content/w81554m2m8760r62/xxlarge1044.gif) ![Acy](/content/w81554m2m8760r62/xxlarge1040.gif) ![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![tscy](/content/w81554m2m8760r62/xxlarge1094.gif) ![Ncy](/content/w81554m2m8760r62/xxlarge1053.gif) ![Ncy](/content/w81554m2m8760r62/xxlarge1053.gif) ![ycy](/content/w81554m2m8760r62/xxlarge1099.gif) ![Dcy](/content/w81554m2m8760r62/xxlarge1044.gif) ![Acy](/content/w81554m2m8760r62/xxlarge1040.gif) ![Ncy](/content/w81554m2m8760r62/xxlarge1053.gif) ![Ncy](/content/w81554m2m8760r62/xxlarge1053.gif) ![ycy](/content/w81554m2m8760r62/xxlarge1099.gif) ![Ocy](/content/w81554m2m8760r62/xxlarge1054.gif) ![tcy](/content/w81554m2m8760r62/xxlarge1090.gif) ![Ncy](/content/w81554m2m8760r62/xxlarge1053.gif) ![Ocy](/content/w81554m2m8760r62/xxlarge1054.gif) ![scy](/content/w81554m2m8760r62/xxlarge1089.gif) ![Icy](/content/w81554m2m8760r62/xxlarge1048.gif) ![tcy](/content/w81554m2m8760r62/xxlarge1090.gif) ![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![lcy](/content/w81554m2m8760r62/xxlarge1083.gif) ![softcy](/content/w81554m2m8760r62/xxlarge1100.gif) ![Ncy](/content/w81554m2m8760r62/xxlarge1053.gif) ![Mcy](/content/w81554m2m8760r62/xxlarge1052.gif) ![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![khcy](/content/w81554m2m8760r62/xxlarge1093.gif) ![Acy](/content/w81554m2m8760r62/xxlarge1040.gif) ![Ncy](/content/w81554m2m8760r62/xxlarge1053.gif) ![Icy](/content/w81554m2m8760r62/xxlarge1048.gif) ![zhcy](/content/w81554m2m8760r62/xxlarge1078.gif) ![Mcy](/content/w81554m2m8760r62/xxlarge1052.gif) ![Rcy](/content/w81554m2m8760r62/xxlarge1056.gif) ![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![Acy](/content/w81554m2m8760r62/xxlarge1040.gif) ![kcy](/content/w81554m2m8760r62/xxlarge1082.gif) ![tscy](/content/w81554m2m8760r62/xxlarge1094.gif) ![Icy](/content/w81554m2m8760r62/xxlarge1048.gif) . ![Dcy](/content/w81554m2m8760r62/xxlarge1044.gif) ![lcy](/content/w81554m2m8760r62/xxlarge1083.gif) ![pcy](/content/w81554m2m8760r62/xxlarge1087.gif) ![Ocy](/content/w81554m2m8760r62/xxlarge1054.gif) ![lcy](/content/w81554m2m8760r62/xxlarge1083.gif) ![Ucy](/content/w81554m2m8760r62/xxlarge1059.gif) ![CHcy](/content/w81554m2m8760r62/xxlarge1063.gif) ![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![Ncy](/content/w81554m2m8760r62/xxlarge1053.gif) ![IOcy](/content/w81554m2m8760r62/xxlarge1025.gif) ![tcy](/content/w81554m2m8760r62/xxlarge1090.gif) ![Icy](/content/w81554m2m8760r62/xxlarge1048.gif) ![kcy](/content/w81554m2m8760r62/xxlarge1082.gif) ![Rcy](/content/w81554m2m8760r62/xxlarge1056.gif) ![Icy](/content/w81554m2m8760r62/xxlarge1048.gif) ![Vcy](/content/w81554m2m8760r62/xxlarge1042.gif) ![ycy](/content/w81554m2m8760r62/xxlarge1099.gif) ![pcy](/content/w81554m2m8760r62/xxlarge1087.gif) ![Rcy](/content/w81554m2m8760r62/xxlarge1056.gif) ![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![Dcy](/content/w81554m2m8760r62/xxlarge1044.gif) ![lcy](/content/w81554m2m8760r62/xxlarge1083.gif) ![Ocy](/content/w81554m2m8760r62/xxlarge1054.gif) ![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![Ncy](/content/w81554m2m8760r62/xxlarge1053.gif) ![tcy](/content/w81554m2m8760r62/xxlarge1090.gif) ![Rcy](/content/w81554m2m8760r62/xxlarge1056.gif) ![Mcy](/content/w81554m2m8760r62/xxlarge1052.gif) ![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![tcy](/content/w81554m2m8760r62/xxlarge1090.gif) ![Ocy](/content/w81554m2m8760r62/xxlarge1054.gif) ![Dcy](/content/w81554m2m8760r62/xxlarge1044.gif) . ![kcy](/content/w81554m2m8760r62/xxlarge1082.gif) ![Acy](/content/w81554m2m8760r62/xxlarge1040.gif) ![CHcy](/content/w81554m2m8760r62/xxlarge1063.gif) ![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![scy](/content/w81554m2m8760r62/xxlarge1089.gif) ![tcy](/content/w81554m2m8760r62/xxlarge1090.gif) ![Vcy](/content/w81554m2m8760r62/xxlarge1042.gif) ![pcy](/content/w81554m2m8760r62/xxlarge1087.gif) ![Rcy](/content/w81554m2m8760r62/xxlarge1056.gif) ![Mcy](/content/w81554m2m8760r62/xxlarge1052.gif) ![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![Rcy](/content/w81554m2m8760r62/xxlarge1056.gif) ![pcy](/content/w81554m2m8760r62/xxlarge1087.gif) ![Rcy](/content/w81554m2m8760r62/xxlarge1056.gif) ![Icy](/content/w81554m2m8760r62/xxlarge1048.gif) ![Vcy](/content/w81554m2m8760r62/xxlarge1042.gif) ![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![Dcy](/content/w81554m2m8760r62/xxlarge1044.gif) ![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![Ncy](/content/w81554m2m8760r62/xxlarge1053.gif) ![Rcy](/content/w81554m2m8760r62/xxlarge1056.gif) ![Acy](/content/w81554m2m8760r62/xxlarge1040.gif) ![zhcy](/content/w81554m2m8760r62/xxlarge1078.gif) ![lcy](/content/w81554m2m8760r62/xxlarge1083.gif) ![Ocy](/content/w81554m2m8760r62/xxlarge1054.gif) ![zhcy](/content/w81554m2m8760r62/xxlarge1078.gif) ![IEcy](/content/w81554m2m8760r62/xxlarge1045.gif) ![Ncy](/content/w81554m2m8760r62/xxlarge1053.gif) ![Icy](/content/w81554m2m8760r62/xxlarge1048.gif) ![Bcy](/content/w81554m2m8760r62/xxlarge1041.gif) ![Icy](/content/w81554m2m8760r62/xxlarge1048.gif) ![kcy](/content/w81554m2m8760r62/xxlarge1082.gif) ![Acy](/content/w81554m2m8760r62/xxlarge1040.gif) ![Rcy](/content/w81554m2m8760r62/xxlarge1056.gif) ![Bcy](/content/w81554m2m8760r62/xxlarge1041.gif) ![Ocy](/content/w81554m2m8760r62/xxlarge1054.gif) ![Acy](/content/w81554m2m8760r62/xxlarge1040.gif) ![tcy](/content/w81554m2m8760r62/xxlarge1090.gif) ![Ncy](/content/w81554m2m8760r62/xxlarge1053.gif) ![Acy](/content/w81554m2m8760r62/xxlarge1040.gif) ![tcy](/content/w81554m2m8760r62/xxlarge1090.gif) ![Rcy](/content/w81554m2m8760r62/xxlarge1056.gif) ![Icy](/content/w81554m2m8760r62/xxlarge1048.gif) .
Nous présentons nos remerciements à la Société Setaram de Lyon pour l'aide matérielle qu'elle nous a apportée au cours de la réalisation de ce travail. |
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