Optical interferometry in phase separated He---He mixture films

We report on interferometric studies of ³He---⁴He liquid mixtures. Anomalous wetting phenomena were observed in phase separated mixture films: the upper ³He-rich phase did not wet the lower ⁴He-rich phase under a small continuous feed of ⁴He atoms to the vapor phase. Instead, under this dynamic situation, floating pools of the ³He-rich phase were stabilized with a contact angle on the order of 10 mrad. In equilibrium, the concentrated ³He-rich phase was found to nucleate uniformly on the free surface, consistent with Antonow's rule.